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The effect of solvent on the reductive coupling reaction between various phenolic reagents and aromatic amines was studied. Phenolic reagents (1-phenyl-2-methylaminopropane, 2,4-dimethyl-aniline, 2-methylaniline, and 2-methylphenol) react with diphenylcarbazide in ethanol to give the corresponding 4-amino-2-methylphenols in good yields. The reaction could be extended to 1-phenyl-1H-pyrrole-2-methylamine, 1-phenyl-2-pyrroleethylamine, 1-phenyl-2-pyrrole-3-methylamine, and 1-phenyl-1,3-dimethylpyrrole. The reaction mechanism of the reaction has been proposed. A quantitative correlation between the rate of the reaction and the basicity of the reaction solution was observed. The stoichiometry of the reaction was determined and it was shown that the reaction occurred via a 2:1 phenolic reagent-phenolic amine complex. The addition of only one equivalent of phenolic amine quenched the organic radical generated from the reductive coupling reaction.Wabi-sabi-san
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